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Research Progress in Conversion of CO2 to Valuable Fuels

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Research Progress in Conversion of CO2 to Valuable Fuels ( research-progress-conversion-co2-valuable-fuels )

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Molecules 2020, 25, 3653 3 of 23 Molecules 2020, 25, x FOR PEER REVIEW 3 of 24 2. Catalytic Reduction of CO2 2.1. Thermal Catalysis Most thermal catalytic conversion of CO2 involves the hydrogenation reaction at relatively low tempMeroastut trheser(m≤5a2l3caKta)ltyotipcrcoodnuvcersuiosenfuolf fCuOelsisnuvcohlvaessCthOe,hmyedtrhoagneen,aatinodnmreeatchtaionnolat[2r8e]l.atSiivnecleyCloOw2 tmemolpeceuraletusraerse(t≤he5r2m3 oKd)ytonapmroicdaullcyeaunsdefcuhlefmueiclsalslyucshtaabsleC, lOar,gmeeatmhaonuen,tasnodf emnetrhgaynaorle[r2e8q].uiSriendceifCO2 2 misoulseecdulaessaasriengthlermeaocdtaynta.mThiceailnlytroadnudcctihoenmoifcoaltlhyerstsaublset,alnacregsewamithohuingthseorfGeinbebrsgfyreaerenrerqguyir(esducihf CasOH2i)saussethdeacsoa-rseiancgtlaenrtewacitlalnmt.akTehethientrhoedrumcotidoynnoafmoitchperoscuebsstaenacsieesrw[2it9h].hInigthheer pGaisbtbfsefwredeecnaedregsy, (gsruecaht atsteHnti)oanshtahsebceoe-nrepaacitdantot twhiellthmearmkealthcaetathlyesrimsodf CynOa2manicdpsriogcneifsiscaenatsipero[g2r9e]s.sIhnasthbeepnasmtafedwe. 2 dVeacraiodues,cgartealtyasttse,ninticolnudhiansgbemeentaplasid(Ctou,thCeot,heetrcm.)alncdatmaleytsaislofxCidOes(aZnndOsi2g, InnifiOc2a,netcp.)ro[g30re–s3s2h]asbweenll 2 masandoev.eVlanraionuos-scizaetadlycsatsa,liynsctlmudeitnagl–moregtanlsic(Cfruam,Ceow,oertkc.s)(aMndOFmse)thaalvoexiadlseos(bZenenOdeIsniOgne,det,cp.)re[3p0a–r3e2d], 2, 2 asndwgerlladasuanlolyvedlevnealnoop-esdiz.ed catalyst metal–organic frameworks (MOFs) have also been designed, prepaRruedn,gatanwdegervaodruaanliltyadnedvecloapuetdh.ors [33] reported a catalyst where Cu nanocrystal (Cu NC) was encapRsuunlgataewdeeivnoranait amnedtacl–ooaurgthaonrics [3f3r]amreepworotrekd aUciaOta-l6y6st w[Zhre6rOe4(COuHn)4a(nBoDcCry)s6,talB(CDuCNC=) w1,a4s- ebnecnazpesnueladtiecdarinboaxmyleattael]–otorgfaonrimc fcramtaelywsotrCkuU⊂iOU-i6O6-[6Z6r, wOh(iOchHc)o(uBlDdCca)t,aBlyDzCe t=he1,g4e-bnenrzaetnioendiocfarmboexthyalantoe]l 6446 tvoiafotrhmechaytadlryostgCenua⊂tUioinO-o6f6,CwOh2i.cFhicgouurled1catsahlyozwesthtehgeesnyenrathtieotnicofpmroectehsasnofolrvianthoerdhyerderdogUeniOat-io6n6ocfryCsOtal. 2 Fstigrucretu1raesfhrowms the sryenatchtieotinc porfoZcerssoxfoidr ean[Zord6Oer4e(OdHU)iO4(−-6C6Oc2r)y1s2]taslesctrouncdtuareyfbroumildthinegreuanctiitosn(SoBf ZUrso) xaindde 2.1. Thermal Catalysis 2 2 nn [BZDrCO.B(OyHus)in(−gCZOr(O)P]rse)4c,onndeaCryubnuailndoincgryusntaitlsw(SaBsUsus)cacnedssBfuDllCy.eBnycuapsisnuglaZtre(dOPinra)n,aonoecCryusntalnUocirOy-s6ta6l, 64 4 212 4 wasashsouwccnesisnfuFlliyguerneca1pbs.uClaut⊂edUiinOa-6n6anwoacsrypsrteacliUseiOly-6p6l,aacesdshonwtnheinCFuigsurrefa1cbe. ,Cyuie⊂lUdinOg-6h6igwhasinpterercfaisceilayl pcolancteadctonbethtweeCeunsCurufaNceC,yaienldinZgrhoixgihdeinSteBrUfasc,iawlchoinchtactobueltdwenensuCreutNhCeraenadctZarnotsxirdeeacShBUths,ewahctiicvhecosiutelds e(Fnisguurereth1ecr)e.aBcytacnotsmrepacrhinthgethacetimveesthiteasn(oFligturneo1vc)e.rBfyrecqoumepnacryin(gTtOheF)moefththaneoClutu⊂rnUoivOe-r6f6recqauteanlycyst(TwOitFh) othfethCeuC/uZ⊂nUOi/OA-l626Oc3atcaltyasltywstitahtthdeifCfeure/ZnntOre/AacltOioncatetamlypsetrattudrifefe(rFenigturereac1tidon),tietmwpearsatfuoruen(dFigthuaret 1tdh)e, 23 iptewrfaosrfmouancdetohfathtehecaptearlfyosrtmexacnecedoefdththeactaotafltyhset Cexuc/eZendOed/Athl2aOt 3ocfatthaelyCsut /aZtnreOla/AtilveOlowcaetarltyesmt apterealtautirvees 23 ◦ l(o

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